Brønsted Acid-Catalyzed Hydroamination of N-Heterocycles to Unactivated Alkenes

Guanzheng Feng, Yisan Shen, Chenghui Sun, Weixiao Ji*, He Huang*, Siping Pang*

*此作品的通讯作者

科研成果: 期刊稿件文章同行评审

摘要

A Brønsted acid-catalyzed hydroamination of unactivated olefins has been developed, enabling the efficient Markovnikov addition of nitrogen heterocycles to olefins. This reaction utilizes a catalytic amount of trifluoroacetic acid (TFA) to produce a diverse array of N-alkyl nitrogen heterocycles. The method is highly scalable, allowing for multigram synthesis, and a novel proton transfer species implicated in olefin activation has been identified.

源语言英语
期刊Asian Journal of Organic Chemistry
DOI
出版状态已接受/待刊 - 2025
已对外发布

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